A team from Nanjing University of Aeronautics and Astronautics (NUAA) has developed an ultrafast laser-assisted in situ hybrid manufacturing process (integrating continuous-wave and ultrafast lasers) to address powder adhesion and slag defects on the sidewalls of high-strength aluminum alloys formed by LPBF. Compared with conventional LPBF, the process reduces side surface roughness from 53.7 μm to 5.2 μm—a 90% decrease—while eliminating balling and powder adhesion. The melt pool transitions from keyhole mode to conduction mode, reducing porosity. The Al₃(Sc,Zr) nanoprecipitates coarsen from 20 nm to 50 nm, and tensile strength increases from approximately 402 MPa to 515 MPa—a 28% improvement—with no significant change in residual stress. This research provides a new pathway for high-precision integrated manufacturing of complex aerospace structures.